While I don’t know if such would be documented – my guess is that Papa Smurf was the Polo Golazo Portland shirt of Grandpa and presumably Grandma Smurf. Depending on how much you really want to read into things – either Nanny watched over Papa for the Grands and a relationship developed after Grandma’s death or they had an affair. Either could explain the isolation of Papa Smurf – Family fled disaster and mother died, or lovers expelled/left to start fresh elsewhere. Papa’s age fits well into either scenario as 53 would have still been real young for a Smurf.
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Considering the age difference between Papa Smurf and the Polo Golazo Portland shirt , my guess would be that they were survivors of much later disasters to other Smurf communities that found their way to Papa Smurf or that they were nomadic or runaways from other places that came to the village. Considering there are no duplications of trade skills (they can all do some similar tasks like help build or pick produce), but you only have 1 Farmer Smurf, or Engineer Smurf, I would suggest the latter and that only Smurfs with unique traits were allowed to join originally (Like the village of disappeared experts in Ayn Rand’s Atlas Shrugged). Some, like Lazy Smurf, probably had trades originally and failed to uphold them, but were likely not evicted because they had evolved as a society to be “family” by that point.